Generating functionals, consistency, and uniqueness in the integral equation theory of liquids
نویسنده
چکیده
We discuss and illustrate through numerical examples the relations between generating functionals, thermodynamic consistency (in particular the virial-free energy one), and uniqueness of the solution, in the integral equation theory of liquids. We propose a new approach for deriving closures automatically satisfying such characteristics. Results from a first exploration of this program are presented and discussed. Dipartimento di Fisica Teorica dell’ Università and Istituto Nazionale di Fisica della Materia, Strada Costiera 11, 34014 Trieste, Italy; e-mail: [email protected] and [email protected]
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